A dynamic two-dimensional heterogeneous model for water gas shift reactors

Title

A dynamic two-dimensional heterogeneous model for water gas shift reactors

Publication Type
Journal Article
Year of Publication
2009
Journal
International Journal of Hydrogen Energy
Number
21
Volume
34
Pagination
8877 – 8891
ISSN
0360-3199
Abstract

A dynamic, heterogeneous, two-dimensional model for packed-bed water gas shift reactors is presented. It can be applied to both high and low temperature shifts, and at scales ranging from industrial (for power plant applications) to small (such as automotive fuel cell applications). The model is suitable for any catalyst for which kinetic data are available, and shows excellent agreement with available experimental data for non-equilibrium conditions. The model is applied to an IGCC-TIGAS polygeneration plant to examine the dynamic behavior of the WGS units. The development of catalyst hot-spots is predicted during start-up or transition between steady states under certain conditions.